For the longest time, Rainbow Six: Siege for me, if I'm watching a competent stack at work, or one with good chemistry who can communicate, it's a joy to watch. Some of those I follow have since branched off into other "competitive" shooters, like Apex and Warzone, which I sometimes watch as well.
Certain ARMA 3 groups or players are also fun to see in action, again though, depends on the players and chemistry. ShackTac does great themed scenarios complete with command structure and whatnot, whereas people like Rimmy and Womble try to be serious, but are more playing it for gaks and giggles.
There's also a German YouTuber named Vade who does a lot of Post Scriptum, Beyond the Wire and Rising Storm 2, whilst not my cuppa tea to play, he makes enjoyable highlight reels, be it commanding a tank, piloting a chopper or sniping people with an AT rifle.
Also the mad rabbit hole that is Fallout New Vegas and Fallout 4 mods, I wouldn't play them myself, so much weird gak out there, but when Mike and Zach from Mikeburnfire play through them, actually worth the watch as they play through it and suffer in our stead. They actually went so far as to play through the train wreck that is Fallout - the Frontier.
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